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The search results do not contain specific information about Inspecteur Zenigata's role or characterization exclusively within the film Lupin III: The Secret of Twilight Gemini. However, the following description synthesizes his general portrayal across the broader Lupin III franchise, which forms the consistent basis for his appearance in that film.

Koichi Zenigata is a middle-aged Japanese inspector working for the International Criminal Police Organization, or Interpol. His entire existence as a law enforcement officer revolves around a single, all-consuming objective: the capture of the legendary thief Arsène Lupin III. This pursuit, which began when he transferred from the Tokyo Metropolitan Police, has become not just a career mandate but the defining purpose of his life. Characterized by an obsessive, single-minded focus that frequently borders on the fanatical, Zenigata is willing to chase Lupin across the globe, often neglecting other responsibilities, his personal well-being, and any semblance of a private life.

Despite his often comedic and bumbling demeanor, particularly in his frantic attempts to corner his quarry, Zenigata is an extraordinarily capable officer. He is widely respected among his peers for his sharp investigative mind and his prior success in dismantling countless criminal organizations long before his fateful encounter with Lupin. His skills are formidable: he is a master of judo and karate, a proficient marksman, and possesses incredible stamina and a high tolerance for pain, which allows him to perform feats of near-superhuman strength and endurance when his obsession is triggered. His signature weapon is a pair of handcuffs attached to a length of rope, which he throws with unerring accuracy in a technique reminiscent of his ancestor, the famous fictional detective Heiji Zenigata. This "handcuff throwing" is a modern evolution of a coin-throwing weapon, and his skill with it is so great that he almost never misses his target.

Zenigata's personality has been portrayed with varying degrees of seriousness throughout the franchise's long history. In his earliest appearances, he was more ruthless, opportunistic, and stern, a morally flexible officer who was primarily focused on results. However, he eventually softened into a more affable, boisterous, and goofy figure, driven by a passionate sense of justice. Core traits that remain constant include an unwavering moral code that makes him resistant to bribery and deeply offended by corruption, as well as a tendency toward impulsiveness and emotional sensitivity. He is known to weep openly when Lupin appears to have died or shows him an unexpected kindness. His personal habits are messy; he never spends much time in one place, so his apartments and desks are notoriously cluttered with papers, empty bottles, and cigarette butts. He does not typically drink or smoke to excess but is known to go on heavy binges when depressed, often when suspended from duty or when his purpose seems lost.

The central dynamic of Zenigata's life is his complex relationship with Lupin III. While their interplay is that of a relentless pursuer and his target, it surpasses a straightforward rivalry to become a profound, symbiotic bond often compared to a "Tom and Jerry" dynamic, where neither character can truly function without the other. An unspoken rule governs their interactions: Zenigata will not kill Lupin, and Lupin will not seriously harm the inspector. Zenigata views it as a personal slight if any other party attempts to capture or kill his nemesis. Conversely, Lupin frequently goes out of his way to save Zenigata from genuine danger or avenge him when he is harmed. Lupin often affectionately calls him "Pops," a nickname Zenigata never truly objects to. This relationship has evolved into a deep, if unacknowledged, mutual respect and even a unique form of friendship. In moments when Lupin is believed to be dead, Zenigata experiences a profound loss of purpose, demonstrating that his identity as a "Lupin chaser" is fundamental to who he is. Despite his permanent record of failure to secure a lasting arrest, Interpol tolerates his methods because his relentless pursuits lead to the incidental capture of a high volume of other dangerous criminals.